Date of Award
T. J. Hammond
Femtosecond, Lasers, Nonlinear optics, Pulse compression, Ultrafast, Z scan
Ultrafast science is a branch of photonics with far reaching applications in and outside the realm of physics. Ultrashort laser pulses on the order of femtoseconds (1 fs = 1 × 10−15 s) are widely used for ultrafast science. Many lasers can produce pulses on the order of 100 fs, with state of the art, high end lasers being capable of producing pulses around 30 fs. However, many experiments require pulses around 10 fs or shorter. Femtosecond pulses are typically generated using spectral broadening via self-phase modulation, followed by dispersion compensation. The most common spectral broadening technique exploits the nonlinear interaction of intense pulses focused into gas-filled hollow-core fibres. More recently, multiple crystal plates have been used to broaden the spectrum while using a self-focusing relay to maintain the beam quality. In this thesis, I research substituting solids and gases with liquid alcohols. By using a series of 1 cm cuvettes filled with 1-decanol, I have compressed a pulse from 83.6 fs down to 31.3 fs with a spectrum capable of supporting 25 fs pulses, all whilst avoiding self-focusing. Liquids have proven to be useful to us due to the ease in which they can be set up and achieve broad spectra as well as their ability to remain intact when exposed to high intensities. In contrast with gases, alcohols provide an inexpensive material for spectral broadening, providing a compact and easy to use setup unhindered by the length of hollow-core fibres. When compared to solids, liquids cannot be damaged permanently as they can easily self-regenerate, allowing a single sample to be reused many times. In this thesis, I show that alcohols provide a compact, inexpensive material for pulse compression that is not susceptible to permanent damage.
Stephen, Jacob A., "Femtosecond Pulse Compression via Self-Phase Modulation in 1-Decanol" (2022). Electronic Theses and Dissertations. 8704.