Faculty members in the Department of Chemistry and Biochemistry have active research programs in a variety of areas, including synthetic inorganic and organic chemistry, materials science, surface science, solid-state chemistry and biological chemistry.

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Submissions from 2012

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Model Iron−Oxo Species and the Oxidation of Imidazole: Insights into the Mechanism of OvoA and EgtB?, Eric Andre Bushnell, Grant B. Fortowsky, and James Gauld

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An assessment of pure, hybrid, meta, and hybrid‐meta GGA density functional theory methods for open‐shell systems: The case of the nonheme iron enzyme 8R–LOX, Eric Andre Bushnell and James Gauld

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Molecular Dynamics Investigation into Substrate Binding and Identity of the Catalytic Base in the Mechanism of Threonyl-tRNA Synthetase, Eric Andre Bushnell, WenJuan Huang, Jorge Llano, and James Gauld

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Stretchable light-emitting electrochemical cells using an elastomeric emissive material, Heather L. Filiatrault, Gyllian C. Porteous, R. Stephen Carmichael, Gregory J.E. Davidson, and Tricia Breen Carmichael

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Alkynedicobalt Complexes in gamma-Carbonyl Cations and Cycloheptynedicobalt Complexes, James R. Green

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Alkynedicobalt Complexes in γ-Carbonyl Cations and Cycloheptynedicobalt Complexes, James R. Green

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Bicatalytic Allylation–Cross-Metathesis Reactions as γ-Carbonyl Cation Equivalents, Jake R. Henkie, Sugadar Dhaliwal, and James R. Green

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Tautomerization in the UDP-Galactopyranose Mutase Mechanism: A DFT-Cluster and QM/MM Investigation, WenJuan Huang and James Gauld

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A Molecular Dynamics (MD) and Quantum Mechanics/Molecular Mechanics (QM/MM) Study on Ornithine Cyclodeaminase (OCD): A Tale of Two Iminiums, Bogdan F. Ion, Eric Andre Bushnell, Phil De Luna, and James Gauld

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Formation of self-assembled monolayers with homogeneously mixed, loosely packed alkyl groups using unsymmetrical dialkyldithiophosphinic acids, Ronan R. San Juan and Tricia Breen Carmichael

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Influence of alkyl chain length on the structure of dialkyldithiophosphinic acid self-assembled monolayers on gold, Ronan R. San Juan, Michael S. Miller, Michael Anthony Ferrato, and Tricia Breen Carmichael

Submissions from 2011

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Dehydrotropylium-Co2(CO)6 Ion. Generation, Reactivity and Evaluation of Cation Stability, Sheida Amiralaei, James Gauld, and James R. Green

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Toxoplasma gondii: Inhibitory Activity and Encystation Effect of Securinine and Pyrrolidine Derivatives on Toxoplasma Growth., Sirinart Ananvoranich

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The first branching point in porphyrin biosynthesis: A systematic docking, molecular dynamics and quantum mechanical/molecular mechanical study of substrate binding and mechanism of uroporphyrinogen‐III decarboxylase, Eric Andre Bushnell, Edvin Erdtman, Jorge Llano, Leif A. Eriksson, and James Gauld

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Computational studies on Schiff-base formation: Implications for the catalytic mechanism of porphobilinogen synthase, Edvin Erdtman, Eric Andre Bushnell, James Gauld, and Leif A. Eriksson

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CO2 Production in the Bromate-1,4-Cyclohexanedione Oscillatory Reaction, Jiamin Feng, James R. Green, Samuel A. Johnson, and Jichang Wang

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Synthesis of ‘Spacer’-Naproxen [2-(6-Methoxybiphenylen-2-yl)propanoic Acid] and -Isonaproxen [2-(7-Methoxybiphenylen-2-yl)propanoic Acid], Juan A. González Gómez, James R. Green, and Peter C. Vollhardt

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The α-Amino Group of the Threonine Substrate as The General Base During tRNA Aminoacylation: A New Version of Substrate-Assisted Catalysis Predicted by Hybrid DFT, WenJuan Huang, Eric Andre Bushnell, Christopher S. Francklyn, and James Gauld

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Vinylogous Nicholas Reactions in the Synthesis of Icetexane, Faveline, and Related Ring Systems, Izabela Kolodziej and James R. Green

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New dialkyldithiophosphinic acid self-assembled monolayers (SAMs): Influence of gold substrate morphology on adsorbate binding and SAM structure, Michael S. Miller, Ronan R.San Juan, Michael Anthony Ferrato, and Tricia Breen Carmichael

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A Sulfonium Cation Intermediate in the Mechanism of Methionine Sulfoxide Reductase B: A DFT Study, Jesse J. Robinet, Hisham Mohammed Mohammed Dokainish, David J. Paterson, and James Gauld

Submissions from 2010

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Silencing of Tachyzoite Enolase 2 Alters Nuclear Targeting of Bradyzoite Enolase 1 in Toxoplasma gondii., Sirinart Ananvoranich

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Intramolecular Nicholas Reactions in the Synthesis of Dibenzocycloheptanes. Synthesis of Allocolchicine NSC 51046 and Analogues and the Formal Synthesis of (−)-Allocolchicine, Sinisa Djurdjevic, Fei Yang, and James R. Green

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Computational Insights into the Mechanism of Porphobilinogen Synthase, Edvin Erdtman, Eric Andre Bushnell, James Gauld, and Leif A. Eriksson

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Neutron diffraction and Vitamin E, T. A. Harroun, D. Marquardt, J. Katsaras, and J. Atkinson

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A DFT study on the catalytic mechanism of UDP-glucose dehydrogenase, WenJuan Huang, Jorge Llano, and James Gauld

Redox Mechanism of Glycosidic Bond Hydrolysis Catalyzed by 6-Phospho-α-glucosidase: A DFT Study, WenJuan Huang, Jorge Llano, and James Gauld

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Location of chlorhexidine in DMPC model membranes: A neutron diffraction study, Ivana Komljenović, Drew Marquardt, Thad A. Harroun, and Edward Sternin

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Cholesterol in unusual places, N. Kučerka, M. P. Nieh, D. Marquardt, T. A. Harroun, S. R. Wassail, and J. Katsaras

Cholesterol in bilayers with PUFA chains: Doping with DMPC or POPC results in sterol reorientation and membrane-domain formation, Norbert Kučerka, Drew Marquardt, Thad A. Harroun, Mu Ping Nieh, Stephen R. Wassall, Djurre H. De Jong, Lars V. Schäfer, Siewert J. Marrink, and John Katsaras

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Templated self-assembly of glass microspheres into ordered two-dimensional arrays under dry conditions, Michael S. Miller, Gregory J.E. Davidson, and Tricia Breen Carmichael

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Selectively metallized polymeric substrates by microcontact printing an aluminum(III) porphyrin complex, Michael S. Miller, Heather L. Filiatrault, Gregory J.E. Davidson, Minmin Luo, and Tricia Breen Carmichael

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Nicholas Reactions in the Construction of Cyclohepta[de]naphthalenes and Cyclohepta[de]naphthalenones. The Total Synthesis of Microstegiol, RAFIQ TAJ and James R. Green

Submissions from 2009

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The functional significance of lipid diversity: Orientation of cholesterol in bilayers is determined by lipid species, Norbert Kučerka, Drew Marquardt, Thad A. Harroun, Mu Ping Nieh, Stephen R. Wassall, and John Katsaras

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A DFT Study of Nucleobase Dealkylation by the DNA Repair Enzyme AlkB, Haining Liu and James Gauld

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Protonation of guanine quartets and quartet stacks: insights from DFT studies, Haining Liu and James Gauld

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Cyclohepta[de]naphthalenes and the Rearranged Abietane Framework of Microstegiol via Nicholas Reaction Chemistry, Rafiq A. Taj, Anusha Abhayawardhana, and James R. Green

Submissions from 2008

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Generation and reactivity of the dehydrotropylium-Co(2)(CO)(6) ion, Sheida Amiralaei and James R. Green

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Substrate-assisted Catalysis in the Aminoacyl Transfer Mechanism of Histidyl−tRNA Synthetase: A Density Functional Theory Study, Haining Liu and James Gauld

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Fabrication of elastomeric wires by selective electroless metallization of poly(dimethylsiloxane), Michael S. Miller, Gregory J.E. Davidson, Brian J. Sahli, Colleen M. Mailloux, and Tricia B. Carmichael

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A Density Functional Theory Investigation on the Mechanism of the Second Half-Reaction of Nitric Oxide Synthase, Jesse J. Robinet, Kyung-Bin Cho, and James Gauld

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DFT Investigation on the Mechanism of the Deacetylation Reaction Catalyzed by LpxC, Jesse J. Robinet and James Gauld

Submissions from 2007

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A Computational Study on the Interaction of the Nitric Oxide Ions NO+ and NO- with the Side Groups of the Aromatic Amino Acids, Jesse J. Robinet, Cristina Baclu, Kyung-Bin Cho, and James Gauld

Submissions from 2006

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Lewis and protic acid mediated Nicholas reactions of 3-acetoxycyclohept-1-en-4-ynedicobalt hexacarbonyl: site selectivity of nucleophile incorporation, Joseph DiMartino and James R. Green

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Density Functional Theory Investigation on the Mechanism of the Hepatitis Delta Virus Ribozyme, Haining Liu, Jesse J. Robinet, Sirinart Ananvoranich, and James Gauld

Submissions from 2005

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Benzocycloheptynedicobalt complexes by intramolecular Nicholas reactions, Y. Ding and James R. Green

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Intramolecular Pauson-Khand reactions of cycloheptynedicobalt complexes, Ahmed B. Mohamed, James R. Green, and Jason Masuda

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Imaging patterns of intensity in topographically directed photolithography, Kateri E. Paul, Tricia L. Breen, Tanja Hadzik, George M. Whitesides, Stephen P. Smith, and Mara Prentiss

Submissions from 2004

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Selective electroless metal deposition using microcontact printing of phosphine-phosphonic acid inks, Tricia Breen Carmichael, Sarah J. Vella, and Ali Afzali

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Mono- and disubstitutions of (hepta-2,5-diyne-1,7-diol) bis(dicobalt) derivatives - Selectivity in Nicholas reactions, Richard Guo, Romelo Gibe, and James R. Green

Submissions from 2003

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Tethered 2+2+2 cycloaddition reactions of cobalt-cycloheptyne complexes, A. B. Mohamed and James R. Green

Submissions from 2002

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An efficient synthesis of symmetrical oligothiophenes: Synthesis and transport properties of a soluble sexithiophene derivative, A. Afzali, T. L. Breen, and C. R. Kagan

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High-performance, solution-processed organic thin film transistors from a novel pentacene precursor, Ali Afzali, Christos D. Dimitrakopoulos, and Tricia L. Breen

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Patterning indium tin oxide and indium zinc oxide using microcontact printing and wet etching, Tricia L. Breen, Peter M. Fryer, Ronald W. Nunes, and Mary E. Rothwell

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Synthesis of cyclophanetetrayne complexes from bis(propargyldicobalt) dication equivalents, R. Gibe and James R. Green

Submissions from 2001

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Cycloheptenyne dicobalt hexacarbonyl complexes by ring closing metathesis, James R. Green

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Patterning organic-inorganic thin-film transistors using microcontact printed templates, C. R. Kagan, T. L. Breen, and L. L. Kosbar

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Tandem 4+3 cycloaddition/nucleophilic trapping reactions of butyne-1,4-diether dicobalt hexacarbonyl complexes, Yafan Lu and James R. Green

Submissions from 2000

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Forming electrical networks in three dimensions by self-assembly, D. H. Gracias, J. Tien, T. L. Breen, C. Hsu, and G. M. Whitesides

Submissions from 1999

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Design and self-assembly of open, regular, 3D mesostructures, Tricia L. Breen, Joe Tien, Scott R.J. Oliver, Tanja Hadzic, and George M. Whitesides

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One step synthesis of [7]metacyclophanediyne complexes from bis(propargyldicobalt) dication equivalents, R. Guo and James R. Green

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4+3 and Fluorinative 4+3 Cycloadditions of Alkyne 1,4-Diether Dicobalt Complexes, M. M. Patel and James R. Green

Submissions from 1998

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Cycloheptyne-cobalt complexes via allylation of stabilized gamma-carbonyl cations, James R. Green

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Maskless photolithography: Embossed photoresist as its own optical element, Kateri E. Paul, Tricia L. Breen, Joanna Aizenberg, and George M. Whitesides

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Crystallization of millimeter-scale objects with use of capillary forces [3], J. Tien, T. L. Breen, and G. M. Whitesides

Submissions from 1997

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Metallacycle transfer routes to main-group phosphacycles, Tricia L. Breen and Douglas W. Stephan

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Combined Ion Mobility/Time-of-Flight Mass Spectrometry Study of Electrospray-Generated Ions, R. Guevremont, K.W. Michael Siu, J. Wang, and L. Ding

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Collision-induced dissociation of 30 m/z unit wide windows of electrospray-generated ions sampled under lens conditions of nominally zero potential gradient, F. Ke, R. Guevremont, and K.W. Michael Siu

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Complexes of silver(I) with peptides and proteins as produced in electrospray mass spectrometry, H. Li, K.W. Michael Siu, R. Guevremont, and J.C.Y. Le Blanc

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Synthesis, Photophysics, and Electrochemistry of Ruthenium(II) Polypyridine Complexes with Crown Ether Pendants, V. W. Yam, V.W. Lee, F. Ke, and K.W. Michael Siu

Submissions from 1996

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Reactivity studies of methylzirconocene phosphide complexes, Tricia L. Breen and Douglas W. Stephan

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Synthesis and reactivity of phosphametallacycles: Sterically induced epimerizations and retrocycloadditions, Tricia L. Breen and Douglas W. Stephan

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Synthesis and reactivity of phosphametallacyclobutenes: Sterically induced [4 + 2] retrocycloadditions, Tricia L. Breen and Douglas W. Stephan

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Zr-E π-bonding in complexes derived from E-H additions to Cp2Zr(P(C6H2-2,4,6-t-Bu3))(PMe 3), Tricia L. Breen and Douglas W. Stephan

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(R)- and (S)-enantioselective lithiation of (arene)tricarbonylchromium acetal complexes with chiral alkyllithiums, M. J. Siwek and James R. Green

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Electrospray tandem mass spectrometry of alkali metal-containing anionic complexes of tripeptide, J. Wang, F. Ke, K.W. Michael Siu, and R. Guevremont

Submissions from 1995

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Phosphinidene Transfer Reactions of the Terminal Phosphinidene Complex Cp2Zr(PC6H2-2,4,6-t-Bu3)(PMe3), Tricia L. Breen and Douglas W. Stephan

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Preparation and certification of a biological reference material (CARP-1) for polychlorinated dibenzo-p-dioxin and dibenzofuran congeners, C. A. Fraser, G.J. Gardner, P.S. Maxwell, and K.W. Michael Siu

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Physico-chemical characterization of metal binding proteins using HPLC-ICP-MS, HPLC-MA-AAS and electrospray-MS, K. A. High, B.A. Methven, J.W. McLaren, and K.W. Michael Siu

Erratum: Early metal mediated P-P bond formation in Cp2M((PR)2) and Cp2M((PR)3) complexes (Inorganic Chemistry (1994) 33, (865-870)), Jianwei Ho, Tricia L. Breen, Andrzej Ozarowski, and Douglas W. Stephan

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Electrospray tandem mass spectrometry of polyoxoanions, T. C. Lau, J. Wang, R. Guevremont, and K.W. Michael Siu

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Propargyl Chlorides as Sources for Cobalt Stabilized γ-Carbonyl Cations, C. Stephen Vizniowski, James R. Green, Tricia L. Breen, and Andrea V. Dalacu

Submissions from 1994

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Early Metal Mediated P-P Bond Formation in Cp2M((PR)2) and Cp2M((PR)3) Complexes, Jianwei Ho, Tricia L. Breen, Andrzej Ozarowski, and Douglas W. Stephan

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Electrospray tandem mass spectrometry of oxo complexes of chromium, manganese and tuthenium, T. C. Lau, J. Wang, K.W. Michael Siu, and R. Guevremont

Submissions from 1993

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Formation and Reactivity of the Early Metal Phosphides and Phosphinidenes Cp*2ZrPR, Cp*2Zr(PR)2, and Cp*2Zr(PR)3, Zhaomin Hou, Tricia L. Breen, and Douglas W. Stephan

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Electrospray mass spectrometry of some proteins and the aqueous solution acid/base equilibrium model in the negative ion detection mode, J.C.Y Le Blanc, R. Guevremont, and K.W. Michael Siu

Submissions from 1992

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Substitution or Nucleophilic Attack by Phosphines on ZrCl4(THF)2, Trida L. Breen and Douglas W. Stephan

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Electrospray mass spectrometry: a study on some aqueous solutions of metal salts, Z. L. Cheng, K.W. Michael Siu, R. Guevremont, and Shiere S. Berman

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Are the electrospray mass spectra of proteins related to their aqueous solution chemistry?, R. Guevremont, K.W. Michael Siu, J.C.Y. Le Blanc, and Shiere S. Berman

Submissions from 1991

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Determination of butyltins in mussel by gas chromatography with flame photometric detection using quartz surface-induced luminescence, G.B. Jiang, P.S. Maxwell, K.W. Michael Siu, and V.T. Luong

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Electrospray mass spectrometry: Application of ion evaporation theory to amino acids, M. Sakairi, A.L. Yergey, K.W. Michael Siu, and J.C.Y. Le Blanc

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Electrospray interfacing for the coupling of ion-exchange and ion-paring chromatography to mass spectrometry, K.W. Michael Siu, R. Guevremont, J.C.Y. Le Blanc, and G.J. Gardner

Submissions from 1990

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Hypercoulometry of the second kind in electron-capture detection, W.A. Aue, K.W. Michael Siu, D. Beauchemin, and Shiere S. Berman

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Applications of ICP-MS in marine analytical chemistry, J.W. McLaren, K.W. Michael Siu, J.W. Lam, and S.N. Willie

Submissions from 1989

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Determination of arsenic species by high-performance liquid chromatography - Inductively coupled plasma mass spectrometry, D. Beauchemin, K.W. Michael Siu, J.W. McLaren, and Shiere S. Berman

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Marine biological reference materials for methylmercury: analytical methodologies used in certification, S.S. Berman, K.W. Michael Siu, P.S. Maxwell, and D. Beauchemin

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Ion-spray mass spectrometry of marine neurotoxins., M.A. Quilliam, B.A. Thomson, G.J. Scott, and K.W. Michael Siu

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Exchange of comments on identification and quantitation of arsenic species in a dogfish muscle reference material for trace elements, Y. Shibata, M. Morita, K.W. Michael Siu, and R.E. Sturgeon

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Ionspray mass spectrometry/mass spectrometry: Quantitation of tributyltin in a sediment reference material for trace metals, K.W. Michael Siu, G.J. Gardner, and Shiere S. Berman

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Extraction of butyltin species and their gas chromatographic determination as chlorides in a sediment certified reference material for trace metals, PACS-1, K.W. Michael Siu, P.S. Maxwell, and Shiere S. Berman